The database includes thermal data analysis for silica-composites that conclude the loading amount of amine adsorbents of each composite as well as each specimen's ability to adsorb CO2. The data repository includes raw data files for: thermogravimetric analysis (TGA) weight loss and CO2 adsorption traces, and Fourier Transform Infrared Spectroscopy (FTIR) spectra?s. For more information see the readme and data documentation. A complete manuscript describing data collection, analysis, and database documentation is to be published. File formats for data include: .txt and .csv.